Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model

Touitou, Jamal and Aiouache, Farid and Burch, Robbie and Roy, Douglas and Hardacre, Christopher and Morgan, Kevin and Sa, Jacinto and Stewart, Caomhan and Stewart, Jonathan and Goguet, Alexandre (2014) Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model. Journal of Catalysis, 319. pp. 239-246. ISSN 0021-9517

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Abstract

This paper reports the detailed description and validation of a fully automated, computer controlled analytical method to spatially probe the gas composition and thermal characteristics in packed bed systems. This method has been designed to limit the invasiveness of the probe, a characteristic assessed using CFD. The thermocouple is aligned with the sampling holes to enable simultaneous recording of the gas composition and temperature profiles. This analysis technique has been validated by studying CO oxidation over a 1% Pt/Al2O3 catalyst. The resultant profiles have been compared with a micro-kinetic model, to further assess the strength of the technique.

Item Type:
Journal Article
Journal or Publication Title:
Journal of Catalysis
Uncontrolled Keywords:
/dk/atira/pure/subjectarea/asjc/1600/1606
Subjects:
?? SPATIALLY RESOLVED PROFILESMICRO-KINETIC MODELCOMUTATIONAL FLUID DYNAMICSCATALYSISPHYSICAL AND THEORETICAL CHEMISTRY ??
ID Code:
76649
Deposited By:
Deposited On:
13 Nov 2015 13:12
Refereed?:
Yes
Published?:
Published
Last Modified:
30 Oct 2023 02:35