Manifestation of LO-LA phonons in Raman scattering in graphene

Ferone, Raffaello and Wallbank, John R. and Zolyomi, Viktor and McCann, Edward and Falko, Vladimir (2011) Manifestation of LO-LA phonons in Raman scattering in graphene. Solid State Communications, 151 (16). pp. 1071-1074. ISSN 0038-1098

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Abstract

We analyze the spectral density of Raman scattering in graphene accompanied by the emission of a pair of LO or LA phonons from the corner of the Brillouin zone. Using a minimal tight-binding model approach, we find that the lineshape of the corresponding Raman signal consists of two peaks with a strongly non-Lorentzian (almost triangular) form with their width and the splitting between the peaks being strongly dependent on the energy of the incoming photon. The asymmetric lineshape is determined by the kinematics of the fully-resonant two-phonon process, and it reflects a strong anisotropy of LO–LA phonons’ dispersion around the Brillouin zone corners.

Item Type:
Journal Article
Journal or Publication Title:
Solid State Communications
Uncontrolled Keywords:
/dk/atira/pure/core/keywords/physics
Subjects:
?? a. graphenea. carbon d. electron–phonon interactions e. raman spectroscopyphysicsmaterials chemistrygeneral chemistrycondensed matter physicschemistry(all)qc physics ??
ID Code:
55862
Deposited By:
Deposited On:
16 Jul 2012 09:28
Refereed?:
Yes
Published?:
Published
Last Modified:
16 Jul 2024 09:06