"APEC Blue":Secondary Aerosol Reductions from Emission Controls in Beijing

Sun, Yele and Wang, Zifa and Wild, Oliver and Xu, Weiqi and Chen, Chen and Fu, Pingqing and Du, Wei and Zhou, Libo and Zhang, Qi and Han, Tingting and Wang, Qingqing and Pan, Xiaole and Zheng, Haitao and Li, Jie and Guo, Xiaofeng and Liu, Jianguo and Worsnop, Douglas R. (2016) "APEC Blue":Secondary Aerosol Reductions from Emission Controls in Beijing. Scientific Reports, 6. ISSN 2045-2322

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Abstract

China implemented strict emission control measures in Beijing and surrounding regions to ensure good air quality during the 2014 Asia-Pacific Economic Cooperation (APEC) summit. We conducted synchronous aerosol particle measurements with two aerosol mass spectrometers at different heights on a meteorological tower in urban Beijing to investigate the variations in particulate composition, sources and size distributions in response to emission controls. Our results show consistently large reductions in secondary inorganic aerosol (SIA) of 61-67% and 51-57%, and in secondary organic aerosol (SOA) of 55% and 37%, at 260 m and ground level, respectively, during the APEC summit. These changes were mainly caused by large reductions in accumulation mode particles and by suppression of the growth of SIA and SOA by a factor of 2-3, which led to blue sky days during APEC commonly referred to as "APEC Blue". We propose a conceptual framework for the evolution of primary and secondary species and highlight the importance of regional atmospheric transport in the formation of severe pollution episodes in Beijing. Our results indicate that reducing the precursors of secondary aerosol over regional scales is crucial and effective in suppressing the formation of secondary particulates and mitigating PM pollution.

Item Type:
Journal Article
Journal or Publication Title:
Scientific Reports
Uncontrolled Keywords:
/dk/atira/pure/subjectarea/asjc/1000
Subjects:
?? POSITIVE MATRIX FACTORIZATIONCHEMICAL SPECIATION MONITORNORTH CHINA PLAINMASS-SPECTROMETERCOLLECTION EFFICIENCIESFORMATION MECHANISMORGANIC AEROSOLSURBAN CANOPYAIR-QUALITYPOLLUTIONGENERAL ??
ID Code:
84532
Deposited By:
Deposited On:
02 Feb 2017 16:40
Refereed?:
Yes
Published?:
Published
Last Modified:
16 Sep 2023 01:19