Determination of carcinoembryonic antigen (CEA) by surface plasmon resonance-enhanced total internal reflection ellipsometry (SPRe-TIRE)

Erkal-Aytemur, Aslı and Şahin, Samet and Üstündağ, Zafer and Mülazımoğlu, İbrahim Ender and Caglayan, Mustafa Oguzhan (2023) Determination of carcinoembryonic antigen (CEA) by surface plasmon resonance-enhanced total internal reflection ellipsometry (SPRe-TIRE). Instrumentation Science and Technology. ISSN 1073-9149

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Abstract

A surface plasmon resonance-enhanced total internal reflection ellipsometric (SPRe-TIRE) aptasensor is reported for the determination of the carcinoembryonic antigen (CEA). A gold nanofilm-coated SF10 glass slide was modified with electrochemical diazonium salt reduction and gold nanoparticles (AuNPs) to form a sensor. Next, a specific aptamer for CEA was immobilized on the AuNPs via self-assembly. The platform was characterized by X-ray photoelectron spectroscopy, ellipsometry, and cyclic voltammetry for each step of the preparation of the sensor. CEA aptamers with different affinities were used. SPRe-TIRE employed total internal reflection geometry and AuNPs to enhance plasmon resonance for the sensitive and selective determination of CEA in human serum. The working range of the aptasensor was from 0.01 to 500 ng/mL with an optimum detection limit of 0.1 pg/mL.

Item Type:
Journal Article
Journal or Publication Title:
Instrumentation Science and Technology
Uncontrolled Keywords:
/dk/atira/pure/subjectarea/asjc/1500/1500
Subjects:
?? aptasensorcarcinoembryonic antigen (cea)cyclic voltammetry (cv)surface plasmon resonance-enhanced total internal reflection ellipsometry (spre-tire)general chemical engineeringinstrumentationgeneral environmental scienceenvironmental science(all)chemical ??
ID Code:
209869
Deposited By:
Deposited On:
14 Nov 2023 02:00
Refereed?:
Yes
Published?:
Published
Last Modified:
16 Jul 2024 12:10