Experimental Study of Steam and Carbon Dioxide Microwave Plasma for Advanced Thermal Treatment Application

Vecten, Simon and Wilkinson, Michael and Martin, Alastair and Dexter, Amos and Bimbo, Nuno and Dawson, Richard and Herbert, Ben (2020) Experimental Study of Steam and Carbon Dioxide Microwave Plasma for Advanced Thermal Treatment Application. Energy, 207. ISSN 0360-5442

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Abstract

Pollution reduction from waste management and energy generation is necessary to mitigate climate change and is one of the major challenges of the 21th century. This can be achieved through the development of innovative energy recovery technologies from biomass and wastes, such as microwave plasma gasification. An envelope of stable CO2 plasma operation is described, by varying working gas flow rate at applied microwave powers between 1 and 6 kW, whereas H2O plasma operation is possible with flow rate ranging from 20 to 50 g/min and microwave powers between 2.5 and 6 kW. The temperature generated in a large chamber connected to the plasma torch is recorded, reaching up to 850°C, showing a heterogeneous temperature distribution. In addition, optical emission spectroscopy measurements provide an insight into plasma chemistry and demonstrate the dissociation of CO2 and H2O molecules at extremely high temperatures of up to 6,300°C assuming local thermodynamic equilibrium. The experimental results demonstrate that the microwave plasma torch provides an ideal environment for gasification with high temperature and very chemically reactive species. This study provides valuable information for the design of microwave plasma gasification reactors with great potential for effective solid feedstock conversion into high quality syngas for energy production.

Item Type:
Journal Article
Journal or Publication Title:
Energy
Additional Information:
This is the author’s version of a work that was accepted for publication in Energy. Changes resulting from the publishing process, such as peer review, editing, corrections, structural formatting, and other quality control mechanisms may not be reflected in this document. Changes may have been made to this work since it was submitted for publication. A definitive version was subsequently published in Energy, 207, 2020 DOI: 10.1016/j.energy.2020.118086
Uncontrolled Keywords:
/dk/atira/pure/subjectarea/asjc/2300/2310
Subjects:
ID Code:
144754
Deposited By:
Deposited On:
16 Jun 2020 09:00
Refereed?:
Yes
Published?:
Published
Last Modified:
27 Sep 2020 05:51